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Author(s):   Brouard, M.; O'Keeffe, P.; Vallance, C.
Title:   Product State Resolved Dynamics of Elementary Reactions
Journal:   J. Phys. Chem. A
Volume:   106
Page(s):   3629 - 3641
Year:   2002
Reference type:   Journal article
Squib:   2002BRO/OKE3629-3641

Reaction:   N2O + ·OH + N2
Reaction order:   2
Rate expression:   no rate data available
Category:  Review
Data type:   Extensive literature review
Comments:   The manuscript reviews the photon-initiated reaction technique and its ability to provide dynamical information about elementary gas-phase bimolecular reactions at the product quantum state-resolved level. The primary focus is on the product angular scattering and rotational angular momentum polarization information that can be obtained from bulb experiments. The review illustrates how particular insight into the reaction mechanism is provided by comparisons with the results of model calculations and with ab initio theoretical predictions. It shows how the experimental measurements have helped provide a critical assessment of the ability of current theory to predict the outcome of simple chemical reactions.

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